1cda1794ff8b4528321f4b23bcd58c5b pmc_26964764.pdf a2aa3db0f62fb4b4bddd58e97b84c0ba2acb4e86 pmc_26964764.pdf e1f3bc64d3b2271c48e8ec85ba6b344c52d19931bad407fcdf6205f99c9189d0 pmc_26964764.pdf Title: Thermal selectivity of intermolecular versus intramolecular reactions on surfaces Subject: Nature Communications 7, (2016). doi:10.1038/ncomms11002 Author: Borja Cirera Creator: Arbortext Advanced Print Publisher 9.0.226/W Producer: Acrobat Distiller 8.1.0 (Windows) CreationDate: Thu Mar 3 17:50:05 2016 CET ModDate: Sat Mar 5 07:25:09 2016 CET Tagged: no UserProperties: no Suspects: no Form: AcroForm JavaScript: no Pages: 8 Encrypted: no Page size: 595.276 x 782.362 pts Page rot: 0 File size: 1349881 bytes Optimized: yes PDF version: 1.6 name type encoding emb sub uni object ID ------------------------------------ ----------------- ---------------- --- --- --- --------- DIPFFJ+AdvOTea1a7398 Type 1C Custom yes yes yes 331 0 DIPFGK+Advsymbol Type 1C Custom yes yes no 339 0 DIPFGL+AdvP4C4E74 Type 1C Custom yes yes yes 340 0 DIPFGM+AdvOTcb88df00 Type 1C Custom yes yes yes 341 0 DIPGPD+Arial-BoldMT Type 1C WinAnsi yes yes no 342 0 DIPHCD+AdvOTf23bb480 Type 1C Custom yes yes yes 343 0 DIPHMB+AdvTTda6f6cb8.B Type 1C Custom yes yes yes 360 0 DIPIGC+AdvOT7d6df7ab.I Type 1C Custom yes yes yes 192 0 DIPIGD+AdvItcSymbol-M Type 1C WinAnsi yes yes no 170 0 DIPIHD+AdvPi2 Type 1C WinAnsi yes yes no 188 0 DIPIHE+AdvPi1 Type 1C WinAnsi yes yes no 195 0 DJAJAP+Helvetica-Bold Type 1C WinAnsi yes yes no 187 0 DJCBHK+AdvOT9bd21c25.I Type 1C Custom yes yes yes 199 0 DIPIEO+AdvOT125c650c Type 1C Custom yes yes yes 185 0 DIPIEP+AdvOT1ef757c0 Type 1C Custom yes yes yes 167 0 DIPIGA+AdvOTb65e897d.B Type 1C Custom yes yes yes 168 0 DIPIGB+AdvEls-ent7 Type 1C WinAnsi yes yes no 190 0 DJDPCF+Helvetica Type 1C WinAnsi yes yes no 203 0 DJECHC+Helvetica-Oblique Type 1C WinAnsi yes yes no 201 0 DKBCEG+AdvP4C4E51 Type 1C Custom yes yes yes 207 0 Jhove (Rel. 1.22.1, 2019-04-17) Date: 2023-02-16 03:03:38 CET RepresentationInformation: pmc_26964764.pdf ReportingModule: PDF-hul, Rel. 1.12.1 (2019-04-17) LastModified: 2018-02-06 09:07:22 CET Size: 1349881 Format: PDF Version: 1.6 Status: Well-Formed and valid SignatureMatches: PDF-hul MIMEtype: application/pdf Profile: Linearized PDF PDFMetadata: Objects: 383 FreeObjects: 1 IncrementalUpdates: 1 DocumentCatalog: PageLayout: SinglePage PageMode: UseNone Outlines: Item: Title: title_link Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@4d3167f4 Children: Item: Title: Results Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@ed9d034 Children: Item: Title: Self-assembly of OETAP precursors on Au(111) Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@6121c9d6 Item: Title: Polymerization of OETAP species Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@87f383f Item: Title: Figure™1Self-assembly of OETAP on Au(111) after deposition at room temperature.(a) High-resolution STM images revealing submolecular features. Black arrows depict the lattice vectors of the rhombic unit cell. Black star shows the close-packed directions o Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@4eb7f003 Children: Item: Title: Transformation of OETAP precursors into phthalocyanines Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@eafc191 Item: Title: Figure™2Surface-confined synthesis of phthalocyanine tapes.The deposition of 0.3 ML of OETAP species (precursors) on Au(111) held at room temperature and subsequent gently annealing at 275thinspdegC affords the formation of phthalocyanine polymers. (a) Lo Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@612fc6eb Item: Title: Figure™3Surface-assisted synthesis and self-assembly of phthalocyanines.The deposition of OETAP species on Au(111) held at 300thinspdegC affords the on-surface chemical transformation of precursors into phthalocyanine species. (a) Long-range STM image, re Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@1060b431 Children: Item: Title: Reaction intermediates during polymerization Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@612679d6 Item: Title: Figure™4Surface-assisted formation of phthalocyanine derivatives after deposition of OETAP precursors on Au(111).(a,e) Large-scale STM images showing the formation of patches of initially reacted molecules coexisting with unreacted species. (b-d) High-res Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@11758f2a Item: Title: Discussion Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@e720b71 Item: Title: Figure™5Proposed reaction mechanisms describing the surface-assisted formation of phthalocyanine polymers and monomers on Au(111).(a) Reaction steps involving STM-imaged intermediates 1-L and 2-L in the phthalocyanine dimer formation (3-L reaction product Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@1b26f7b2 Item: Title: Figure™6Reaction pathway considerations for a model pyrrole molecule on Au(111).(a-c) Monomer cyclization. (d-f) Initial steps of the dimerization process. For both reactions, it is assumed that the ethyl legs have been transformed into ethenyl groups thr Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@491cc5c9 Item: Title: Methods Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@74ad1f1f Children: Item: Title: Experiments Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@6a1aab78 Item: Title: Theory Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@462d5aee Item: Title: GourdonA.On-surface covalent coupling in ultrahigh vacuumAngew. Chem. Int. Ed.47695069532008FrancG.GourdonA.Covalent networks through on-surface chemistry in ultra-high vacuum: state-of-the-art and recent developmentsPhys. Chem. Chem. Phys.131428314292201 Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@69b0fd6f Item: Title: We thank the financial support of the EU (projects ERC Starting Grant CHEMCOMP no 279313, EC FP7-PEOPLE-2011-COFUND AMAROUT II program, EC FP7-PEOPLE-2013-CIG &!QJ;(no. 631396) and FEDER CTQ2014-56295-R), the Spanish Ministerio de Economía y Competitivida Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@757942a1 Item: Title: ACKNOWLEDGEMENTS Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@4a87761d Item: Title: Author contributions Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@66d1af89 Item: Title: Additional information Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@8646db9 Info: Title: Thermal selectivity of intermolecular versus intramolecular reactions on surfaces Author: Borja Cirera Subject: Nature Communications 7, (2016). doi:10.1038/ncomms11002 Creator: Arbortext Advanced Print Publisher 9.0.226/W 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FontFile3: true Encoding: WinAnsiEncoding Font: BaseFont: DIPIHD+AdvPi2 FontSubset: true FirstChar: 121 LastChar: 121 FontDescriptor: FontName: DIPIHD+AdvPi2 Flags: Serif, Nonsymbolic FontBBox: 16, -335, 981, 833 FontFile3: true Encoding: WinAnsiEncoding Font: BaseFont: DIPIGB+AdvEls-ent7 FontSubset: true FirstChar: 66 LastChar: 66 FontDescriptor: FontName: DIPIGB+AdvEls-ent7 Flags: Nonsymbolic FontBBox: 51, -322, 1177, 843 FontFile3: true Encoding: WinAnsiEncoding XMP: application/pdf doi:10.1038/ncomms11002 Borja Cirera Nelson Giménez-Agulló Jonas Björk Francisco Martínez-Peña Alberto Martin-Jimenez Jonathan Rodriguez-Fernandez Ana M Pizarro Roberto Otero José M. Gallego Pablo Ballester José R. Galan-Mascaros David Ecija Nature Communications 7, (2016). doi:10.1038/ncomms11002 Nature Publishing Group © 2016 Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. Thermal selectivity of intermolecular versus intramolecular reactions on surfaces Acrobat Distiller 8.1.0 (Windows) © 2016 Nature Publishing Group, a division of Macmillan Publishers Limited. 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