cf10dc3d9de85748166e6e7aacdc9395 pmc_26948987.pdf acae1d6fe88b4d5748e3532b0874bf614bc4fca6 pmc_26948987.pdf c8cfe1639ebd0d6ac11c1c95558be78850fcd9715d6071b456e5f3d73f5f9201 pmc_26948987.pdf Title: High-performance thermoelectric nanocomposites from nanocrystal building blocks Subject: Nature Communications 7, (2016). doi:10.1038/ncomms10766 Author: Maria Ibáñez Creator: Arbortext Advanced Print Publisher 9.0.226/W Producer: Acrobat Distiller 8.1.0 (Windows) CreationDate: Mon Feb 29 09:30:50 2016 CET ModDate: Mon Feb 29 12:18:27 2016 CET Tagged: no UserProperties: no Suspects: no Form: AcroForm JavaScript: no Pages: 7 Encrypted: no Page size: 595.276 x 782.362 pts Page rot: 0 File size: 2216205 bytes Optimized: yes PDF version: 1.6 name type encoding emb sub uni object ID ------------------------------------ ----------------- ---------------- --- --- --- --------- ALCMPB+AdvOTea1a7398 Type 1C Custom yes yes yes 300 0 ALCMPC+AdvTimes-i Type 1C Custom yes yes yes 301 0 ALCNAD+AdvOTcb88df00 Type 1C Custom yes yes yes 309 0 ALCNFC+Arial-BoldMT Type 1C WinAnsi yes yes no 310 0 ALCNHC+AdvOTf23bb480 Type 1C Custom yes yes yes 311 0 ALCOCO+AdvTTda6f6cb8.B Type 1C Custom yes yes yes 321 0 ALCONB+AdvPi1 Type 1C WinAnsi yes yes no 138 0 ALCOPB+AdvOTb65e897d.B Type 1C Custom yes yes yes 139 0 ALDKDN+Helvetica Type 1C WinAnsi yes yes no 127 0 ALDLIG+Helvetica-Oblique Type 1C WinAnsi yes yes no 128 0 ALCOLM+AdvOT125c650c Type 1C Custom yes yes yes 154 0 ALCOLN+AdvOT1ef757c0 Type 1C Custom yes yes yes 155 0 ALCOLO+AdvOT7d6df7ab.I Type 1C Custom yes yes yes 144 0 ALCOMP+AdvPi2 Type 1C WinAnsi yes yes no 145 0 ALCONA+AdvP4C4E74 Type 1C Custom yes yes yes 149 0 ALIMGG+Symbol Type 1C Custom yes yes yes 173 0 ALIMGH+Helvetica-Bold Type 1C WinAnsi yes yes no 159 0 ALJMCH+MathPackTen Type 1C Custom yes yes yes 175 0 ALJOCM+AdvOT9bd21c25.I Type 1C Custom yes yes yes 176 0 ALKMOC+AdvEls-ent5 Type 1C WinAnsi yes yes no 184 0 ALKMOD+Advsymbol Type 1C Custom yes yes no 183 0 ALMIEM+AdvEls-ent7 Type 1C WinAnsi yes yes no 185 0 Jhove (Rel. 1.22.1, 2019-04-17) Date: 2023-02-16 02:53:34 CET RepresentationInformation: pmc_26948987.pdf ReportingModule: PDF-hul, Rel. 1.12.1 (2019-04-17) LastModified: 2018-02-06 09:07:43 CET Size: 2216205 Format: PDF Version: 1.6 Status: Well-Formed and valid SignatureMatches: PDF-hul MIMEtype: application/pdf Profile: Linearized PDF PDFMetadata: Objects: 348 FreeObjects: 1 IncrementalUpdates: 1 DocumentCatalog: PageLayout: SinglePage PageMode: UseNone Outlines: Item: Title: title_link Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@4d3167f4 Children: Item: Title: Results Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@ed9d034 Children: Item: Title: PbS-Ag nanocomposites Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@6121c9d6 Item: Title: Figure™1Bottom-up Design.Bottom-up assembly process to produce PbS-Ag TE nanocomposites from the assembly of PbS (blue) and Ag (red) NCs, and the corresponding band alignment of the resulting nanocomposite Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@87f383f Children: Item: Title: Thermoelectric properties Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@4eb7f003 Item: Title: Figure™2Structural and compositional characterization of initial NCs and resulting PbS-Ag 4.4thinspmolpercnt nanocomposite.TEM micrographs of (a) PbS and (b) Ag NCs; (c) HAADF-STEM micrograph and elemental EDX maps; and (d) HRTEM micrograph of the PbS-Ag Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@eafc191 Item: Title: Figure™3Thermoelectric characterization of PbS-Ag nanocomposites.Temperature dependence of the (a) electrical conductivity, sgr; (b) Seebeck coefficient, S; (c) thermal conductivity, kappa; and (d) power factor, PF. Error bars were estimated from the repe Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@612fc6eb Item: Title: Discussion Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@1060b431 Item: Title: Figure™4Figure of merit and schematic representation of the electron energy band alignment.(a) Figure of merit, ZT, of PbS and PbS-Ag pellets; (b) band alignment in PbS-Ag nanocomposite with a larger amount of Ag and flat bands across the whole PbS domain Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@612679d6 Item: Title: Methods Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@11758f2a Children: Item: Title: Nanocomposite preparation Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@e720b71 Item: Title: Figure™5Theoretical calculations.(a) Band alignment at the Ag-PbS interface considering bulk Ag and bulk PbS at 300thinspK. The Fermi level is pinned at -4.4thinspeV (silver work function). Electrons in PbS experience a well, as marked, when going to the Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@1b26f7b2 Item: Title: Figure™6Electrical properties of PbS nanomaterials with different doping strategies.(a) sgr and (b) S of x molpercnt PbS (x=1.5, 3.0, 4.5 and 6.0) doped with Cl (open symbols) compared with pure PbS (0.0thinspmol percnt) and PbS-Ag (4.4thinspmolpercnt). ( Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@491cc5c9 Children: Item: Title: Structural characterization Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@74ad1f1f Item: Title: Thermoelectric characterization Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@6a1aab78 Item: Title: BellL. E.Cooling, heating, generating power, and recovering waste heat with thermoelectric systemsScience321145714612008VineisC. J.ShakouriA.MajumdarA.KanatzidisM. G.Nanostructured thermoelectrics: big efficiency gains from small featuresAdv. Mater.223970 Destination: edu.harvard.hul.ois.jhove.module.pdf.PdfSimpleObject@462d5aee Item: Title: At IREC, work was supported by European Regional Development Funds and the Framework 7 program under project UNION (FP7-NMP 310250). M.I. and S.O. thank AGAUR for their Beatriu i Pinós post-doctoral grant (2013 BP-A00344) and the PhD grant, respectively. 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Kovalenko Andreu Cabot Nature Communications 7, (2016). doi:10.1038/ncomms10766 Nature Publishing Group © 2016 Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. High-performance thermoelectric nanocomposites from nanocrystal building blocks Acrobat Distiller 8.1.0 (Windows) © 2016 Nature Publishing Group, a division of Macmillan Publishers Limited. 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