fd97445f492abe4c1e34d65477621a9f pmc_33801091.pdf 40a701bd9c5e6025990147fd650beebf3fa34274 pmc_33801091.pdf 27a40c1f5ed160ba790c971ff8365b12381e28960771e33025bf14cc220bcbe3 pmc_33801091.pdf Title: Formation of Nickel Oxide Nanocuboids in Ferromagnetic La2Ni1-xMn1+xO6 Subject: The control of the spontaneous formation of nanostructures at the surface of thin films is of strong interest in many different fields, from catalysts to microelectronics, because surface and interfacial properties may be substantially enhanced. Here, we analyze the formation of nickel oxide nanocuboids on top of La2Ni1-xMn1+xO6 double perovskite ferromagnetic thin films, epitaxially grown on SrTiO3 (001) substrates by radio-frequency (RF) magnetron sputtering. We show that, by annealing the films at high temperature under high oxygen partial pressure, the spontaneous segregation of nanocuboids is enhanced. The evolution of the structural and magnetic properties of the films is studied as a function of the annealing treatments at different temperatures. It is shown that the formation of NiOx nanocuboids leads to a nanostructured film surface with regions of locally different electrical transport characteristics. Keywords: ferromagnetic double perovskite; spontaneous formation of NiOx nanocuboids; local transport properties Author: Monica Bernal-Salamanca, Zorica Konstantinović, Carlos Frontera, Víctor Fuentes, Alberto Pomar, Lluis Balcells and Benjamín Martínez Creator: LaTeX with hyperref Producer: pdfTeX-1.40.21 CreationDate: Sun Mar 21 10:41:09 2021 CET ModDate: Sun Mar 21 11:00:18 2021 CET Custom Metadata: no Metadata Stream: no Tagged: no UserProperties: no Suspects: no Form: none JavaScript: no Pages: 13 Encrypted: no Page size: 595.276 x 841.89 pts (A4) Page rot: 0 File size: 6061633 bytes Optimized: no PDF version: 1.7 name type encoding emb sub uni object ID ------------------------------------ ----------------- ---------------- --- --- --- --------- WLENKM+VnURWPalladioL-Bold Type 1 Custom yes yes no 10 0 SQEGTJ+VnURWPalladioL Type 1 Custom yes yes no 15 0 YTMYQC+URWPalladioL-Ital Type 1 Custom yes yes no 19 0 BBKFEQ+URWPalladioL-Bold Type 1 Custom yes yes no 24 0 HYYHEA+CMBSY10 Type 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IncrementalUpdates: 0 DocumentCatalog: PageLayout: SinglePage PageMode: UseNone Outlines: Item: Title: Introduction Destination: section.1 Item: Title: Materials and Methods Destination: section.2 Item: Title: Results and Discussion Destination: section.3 Item: Title: Conclusions Destination: section.4 Item: Title: Destination: section.A. Item: Title: Destination: section.B. Item: Title: References Destination: specialtable.caption.12 Info: Title: Formation of Nickel Oxide Nanocuboids in Ferromagnetic La2Ni1-xMn1+xO6 Author: きはのどっち〠あづひのちぬ〭こちぬちねちのっち〬〠ずはひどっち〠かはのびぴちのぴどのはぶどㄇ〬〠ぃちひぬはび〠うひはのぴづひち〬〠ざロっぴはひ〠うふづのぴづび〬〠ぁぬぢづひぴは〠ぐはねちひ〬〠がぬふどび〠あちぬっづぬぬび〠ちのつ〠あづのなちねロの〠きちひぴロのづぺ Subject: The control of the spontaneous formation of nanostructures at the surface of thin films is of strong interest in many different fields, from catalysts to microelectronics, because surface and interfacial properties may be substantially enhanced. Here, we analyze the formation of nickel oxide nanocuboids on top of La2Ni1-xMn1+xO6 double perovskite ferromagnetic thin films, epitaxially grown on SrTiO3 (001) substrates by radio-frequency (RF) magnetron sputtering. We show that, by annealing the films at high temperature under high oxygen partial pressure, the spontaneous segregation of nanocuboids is enhanced. The evolution of the structural and magnetic properties of the films is studied as a function of the annealing treatments at different temperatures. It is shown that the formation of NiOx nanocuboids leads to a nanostructured film surface with regions of locally different electrical transport characteristics. 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