a421b970bc9f94d6fc27e72ee7d34a08 pmc_34062755.pdf f9e4b7953a94a918edf2459a76254d7964a9dbe4 pmc_34062755.pdf 26d16dd609d1bca7373b2cced22ee3cb6e0f19edec9b66474030ac4056ba5c7b pmc_34062755.pdf Title: Carbocycle-Based Organogelators: Influence of Chirality and Structural Features on Their Supramolecular Arrangements and Properties Subject: The rational design and engineer of organogel-based smart materials and stimuli-responsive materials with tuned properties requires the control of the non-covalent forces driving the hierarchical self-assembly. Chirality, as well as cis/trans relative configuration, also plays a crucial role promoting the morphology and characteristics of the aggregates. Cycloalkane derivatives can provide chiral chemical platforms allowing the incorporation of functional groups and hydrophobic structural units able for a convenient molecular stacking leading to gels. Restriction of the conformational freedom imposed by the ring strain is also a contributing issue that can be modulated by the inclusion of flexible segments. In addition, donor/acceptor moieties can also be incorporated favoring the interactions with light or with charged species. This review offers a perspective on the abilities and properties of carbocycle-based organogelators starting from simple cycloalkane derivatives, which were the key to establish the basis for an effective self-assembling, to sophisticated polycyclic compounds with manifold properties and applications. Keywords: low-molecular-weight organogelators; cycloalkanes; cholesterol-based organogelators; chirality; stimuli-responsive materials; self-healing gels Author: Rosa M. 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