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1.
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9 p, 357.9 KB |
Systematic study of the impact of MOF densification into tablets on textural and mechanical properties
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Dhainaut, Jérémy (Université Claude Bernard Lyon 1) ;
Camur, Ceren (Institut Català de Nanociència i Nanotecnologia) ;
Troyano, Javier (Institut Català de Nanociència i Nanotecnologia) ;
Legrand, Alexandre (Institut Català de Nanociència i Nanotecnologia) ;
Canivet, J. (Université Claude Bernard Lyon 1) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Reinsch, Helge (MOFapps) ;
Farrusseng, David (Université Claude Bernard Lyon 1)
Four different metal-organic framework powders (UiO-66, UiO-66-NH, UiO-67, and HKUST-1) were shaped into tablets. The effect of the applied pressure on porous properties, mechanical resistance and tablet bulk density is reported. [...]
2017 -  10.1039/c7ce00338b
CrystEngComm, Vol. 19, issue 29 (August 2017) , p. 4211-4218
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2.
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Spray-drying synthesis of MOFs, COFs, and related composites
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Troyano, Javier (Institut Català de Nanociència i Nanotecnologia) ;
Çamur, Ceren (Institut Català de Nanociència i Nanotecnologia) ;
Garzon-Tovar, Luis (Institut Català de Nanociència i Nanotecnologia) ;
Carné-Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Conspectus: Metal-organic frameworks (MOFs) and covalent organic frameworks (COFs) are among the most attractive porous materials today. They exhibit outstanding porosity for countless applications such as gas storage, CO2 capture, gas separation, sensing, drug delivery, and catalysis. [...]
2020 - 10.1021/acs.accounts.0c00133
Accounts of chemical research, Vol. 53, issue 6 (June 2020) , p. 1206-1217
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3.
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8 p, 1.0 MB |
Net-clipping : an approach to deduce the topology of metal-organic frameworks built with zigzag ligands
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Ortín-Rubio, Borja (Institut Català de Nanociència i Nanotecnologia) ;
Ghasempour, Hosein (Tarbiat Modares University. Department of Chemistry) ;
Guillerm, Vincent (Institut Català de Nanociència i Nanotecnologia) ;
Morsali, Ali (Tarbiat Modares University. Department of Chemistry) ;
Juanhuix, Judith (ALBA Laboratori de Llum de Sincrotró) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Herein we propose a new approach for deducing the topology of metal-organic frameworks (MOFs) assembled from organic ligands of low symmetry, which we call net-clipping. It is based on the construction of nets by rational deconstruction of edge-transitive nets comprising higher-connected molecular building blocks (MBBs). [...]
2020 - 10.1021/jacs.0c03404
Journal of the American Chemical Society, Vol. 142, issue 20 (May 2020) , p. 9135-9140
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4.
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20 p, 1.7 MB |
Biomimetic synthesis of sub-20 nm covalent organic frameworks in water
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Franco, Carlos (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Rodríguez-San-Miguel, David (IFIMAC - Condensed Matter Physics Center) ;
Sorrenti, Alessandro (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Sevim, Semih (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Pons, Ramon (Institut de Química Avançada de Catalunya) ;
Platero-Prats, Ana Eva (IFIMAC - Condensed Matter Physics Center) ;
Pavlovic, Marko (Max-Planck Institute of Colloids and Interfaces. Department of Colloid Chemistry) ;
Szilágyi, Istvan (University of Szeged. Department of Physical Chemistry and Materials Science) ;
Ruiz Gonzalez, M. Luisa (Universidad Complutense de Madrid. Departamento de Quĺmica Inorgánica) ;
González-Calbet, José M. (Universidad Complutense de Madrid. Departamento de Quĺmica Inorgánica) ;
Bochicchio, Davide (University of Applied Sciences and Arts of Southern Switzerland. Department of Innovative Technologies) ;
Pesce, Luca (University of Applied Sciences and Arts of Southern Switzerland. Department of Innovative Technologies) ;
Pavan, Giovanni M. (University of Applied Sciences and Arts of Southern Switzerland. Department of Innovative Technologies) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Cano-Sarabia, Mary (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Pané, Salvador (ETH Zurich. Multi-Scale Robotics Lab) ;
De Mello, Andrew J. (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Zamora, Felix (IFIMAC - Condensed Matter Physics Center) ;
Puigmarti-Luis, Josep (ETH Zurich. Department of Chemistry and Applied Biosciences)
Covalent organic frameworks (COFs) are commonly synthesized under harsh conditions yielding unprocessable powders. Control in their crystallization process and growth has been limited to studies conducted in hazardous organic solvents. [...]
2020 - 10.1021/jacs.9b12389
Journal of the American Chemical Society, Vol. 142, issue 7 (Feb. 2020) , p. 3540-3547
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5.
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23 p, 1.3 MB |
Tuning the supramolecular isomerism of MOF-74 by controlling the synthesis conditions
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Gheorghe, Andreea (Van't Hoff Institute for Molecular Sciences) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Van Der Vlugt, Jarl Ivar (Van't Hoff Institute for Molecular Sciences) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Tanase, Stefania (Van't Hoff Institute for Molecular Sciences)
Supramolecular isomerism of metal-organic frameworks (MOFs) is known for several MOF structures, having direct implications on the properties of these materials. Although the synthesis of MOF isomers is mainly serendipitous in nature, achieving controlled formation of a target framework is highly relevant for practical applications. [...]
2019 - 10.1039/c9dt01572h
Dalton transactions, Vol. 48, issue 27 (July 2019) , p. 10043-10050
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6.
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10 p, 1.1 MB |
Switching acidic and basic catalysis through supramolecular functionalization in a porous 3D covalent imine-based material
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Luis-Barrerra, Javier (Universidad Autónoma de Madrid. Departamento de Química Orgànica) ;
Cano, Rafael (Universidad Autónoma de Madrid. Departamento de Química Inorgànica) ;
Imani-Shakibaei, Ghazaleh (Universidad Autónoma de Madrid. Departamento de Química Orgànica) ;
Heras-Domingo, Javier (Universitat Autònoma de Barcelona. Departament de Química) ;
Pérez-Carvajal, Javier (Institut Català de Nanociència i Nanotecnologia) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Solans Monfort, Xavier (Universitat Autònoma de Barcelona. Departament de Química) ;
Aleman Lara, Jose Julian (Universidad Autónoma de Madrid. Departamento de Química Orgànica) ;
Mas Balleste, Ruben (Universidad Autónoma de Madrid. Departamento de Química Inorgànica)
Non-covalent inclusion of small acid and base molecules (CHCOOH and NEt) in an imine structure based on micrometre COF-300 crystals and amorphous nanoparticles results in the facile modulation of their acid-base properties. [...]
2019 - 10.1039/c9cy01527b
Catalysis science & technology, Vol. 9, issue 21 (Nov. 2019) , p. 6007-6014
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7.
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26 p, 2.5 MB |
Supramolecular fullerene sponges as catalytic masks for regioselective functionalization of C60
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Fuertes-Espinosa, Carles (Universitat de Girona. Departament de Química) ;
García Simón, Cristina (Universitat de Girona. Departament de Química) ;
Pujals Crusat, Míriam (Universitat de Girona. Departament de Química) ;
Garcia-Borràs, Marc (Universitat de Girona. Departament de Química) ;
Gómez, Laura (Universitat de Girona. Serveis Tècnics de Recerca) ;
Parella Coll, Teodor (Universitat Autònoma de Barcelona. Departament de Química) ;
Juanhuix, Judith (ALBA Laboratori de Llum de Sincrotró) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Costas, Miquel (Universitat de Girona. Departament de Química) ;
Ribas, Xavi (Universitat de Girona. Departament de Química)
Isomer-pure poly-functionalized fullerenes are required to boost the development of fullerene chemistry in all fields. On a general basis, multi-adduct mixtures with uncontrolled regioselectivity are obtained, and the use of chromatographic purification is prohibitively costly and time consuming, especially in the production of solar cells. [...]
2020 - 10.1016/j.chempr.2019.10.010
Chem, Vol. 6, issue 1 (Jan. 2020) , p. 169-186
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8.
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9 p, 1.4 MB |
Highly strained, radially π-conjugated porphyrinylene nanohoops
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Xu, Youzhi (University of Ulm. Institute of Organic Chemistry) ;
Gsänger, Sebastian (Friedrich-Alexander-Universität Erlangen-Nürnberg. Interdisciplinary Center for Molecular Materials) ;
Minameyer, Martin B. (Friedrich-Alexander University Erlangen-Nürnberg. Department of Chemistry and Pharmacy) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Shyshov, Oleksandr (University of Ulm. Institute of Organic Chemistry) ;
Schwer, Fabian (University of Ulm. Institute of Organic Chemistry) ;
Ribas, Xavi (Universitat de Girona. Departament de Química) ;
Drewello, Thomas (Friedrich-Alexander University Erlangen-Nürnberg. Department of Chemistry and Pharmacy) ;
Meyer, Bernd (Friedrich-Alexander-Universität Erlangen-Nürnberg. Interdisciplinary Center for Molecular Materials) ;
Von Delius, M. (University of Ulm. Institute of Organic Chemistry)
Small π-conjugated nanohoops are difficult to prepare, but offer an excellent platform for studying the interplay between strain and optoelectronic properties, and, increasingly, these shape-persistent macrocycles find uses in host-guest chemistry and self-assembly. [...]
2019 - 10.1021/jacs.9b08584
Journal of the American Chemical Society, Vol. 141, issue 46 (Nov. 2019) , p. 18500-18507
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9.
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Green synthesis of imine-based covalent organic frameworks in water
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Martín-Illán, Jesús A. (Universidad Autónoma de Madrid. Departamento de Química Inorgánica) ;
Rodríguez-San-Miguel, David (Universidad Autónoma de Madrid. Departamento de Química Inorgánica) ;
Franco, Carlos (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Puigmarti-Luis, Josep (ETH Zurich. Department of Chemistry and Applied Biosciences) ;
Zamora, Félix (Instituto Madrileño de Estudios Avanzados en Nanociencia)
Dynamic covalent bonds have been advantageously used to direct the synthesis of crystalline porous covalent organic frameworks (COFs). Unlike the standard synthetic protocols that involve harsh conditions, this work provides a high-yield "one-pot"green synthesis of imine-based COFs in water. [...]
2020 - 10.1039/d0cc02033h
Chemical communications, Vol. 56, issue 49 (June 2020) , p. 6704-6707
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10.
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17 p, 754.5 KB |
Template-free, surfactant-mediated orientation of self-assembled supercrystals of metal-organic framework particles
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Avci, Civan (Institut Català de Nanociència i Nanotecnologia) ;
Liu, Yang (Institut Català de Nanociència i Nanotecnologia) ;
Pariente, Jose Angel (Instituto de Ciencia de Materiales de Madrid) ;
Blanco, Alvaro (Instituto de Ciencia de Materiales de Madrid) ;
Lopez, Cefe (Instituto de Ciencia de Materiales de Madrid) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Mesoscale self-assembly of particles into supercrystals is important for the design of functional materials such as photonic and plasmonic crystals. However, while much progress has been made in self-assembling supercrystals adopting diverse lattices and using different types of particles, controlling their growth orientation on surfaces has received limited success. [...]
2019 - 10.1002/smll.201902520
Small, Vol. 15, issue 31 (Aug. 2019) , art. 1902520
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