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4 p, 134.6 KB Single-molecule pump-probe detection resolves ultrafast pathways in individual and coupled quantum systems / van Dijk, Erik M. H. P. (Institute for Nanotechnology (Enschede, Països Baixos)) ; Hernando Campos, Jordi (Institute for Nanotechnology (Enschede, Països Baixos)) ; García López, Juan José (Institute for Nanotechnology (Enschede, Països Baixos)) ; Crego Calama, Mercedes (Institute for Nanotechnology (Enschede, Països Baixos)) ; Reinhoudt, David N. (Institute for Nanotechnology (Enschede, Països Baixos)) ; Kuipers, Laurens (Institute for Nanotechnology (Enschede, Països Baixos)) ; García Parajó, María F.. (Institute for Nanotechnology (Enschede, Països Baixos)) ; van Hulst, Niek F.. (Institute for Nanotechnology (Enschede, Països Baixos))
We report the first experimental study of individual molecules with femtosecond time resolution using a novel ultrafast single-molecule pump-probe method. A wide range of relaxation times from below 100 up to 400 fs is found, revealing energy redistribution over different vibrational modes and phonon coupling to the nanoenvironment. [...]
2005 - 10.1103/PhysRevLett.94.078302
Physical review letters, Vol. 94, Issue 7 (February 2005) , p. 78302  
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