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8 p, 2.1 MB Molecular engineering to tune the ligand environment of atomically dispersed nickel for efficient alcohol electrochemical oxidation / Liang, Zhifu (Institut Català de Nanociència i Nanotecnologia) ; Jiang, Daochuan (Anhui University. School of Chemistry and Chemical Engineering) ; Wang, Xiang (Institut de Recerca en Energia de Catalunya) ; Shakouri, Mohsen (Canadian Light Source) ; Zhang, Ting (Institut Català de Nanociència i Nanotecnologia) ; Li, Zhongjun (Hefei University of Technology. School of Physics.) ; Tang, PengYi (Shanghai Institute of Microsystem and Information Technology) ; Llorca, Jordi (Universitat Politècnica de Catalunya. Departament d'Enginyeria Química) ; Liu, Lijia (Western University. Department of Chemistry) ; Yuan, Yupeng (Anhui University. School of Chemistry and Chemical Engineering) ; Heggen, Marc (Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (Jülich, Alemanya)) ; Dunin-Borkowski, Rafal E. (Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (Jülich, Alemanya)) ; Morante, Joan Ramon (Institut de Recerca en Energia de Catalunya) ; Cabot, Andreu (Institució Catalana de Recerca i Estudis Avançats) ; Arbiol i Cobos, Jordi (Institut Català de Nanociència i Nanotecnologia)
Atomically dispersed metals maximize the number of catalytic sites and enhance their activity. However, their challenging synthesis and characterization strongly complicates their optimization. Here, the aim is to demonstrate that tuning the electronic environment of atomically dispersed metal catalysts through the modification of their edge coordination is an effective strategy to maximize their performance. [...]
2021 - 10.1002/adfm.202106349
Advanced functional materials, Vol. 31, issue 51 (Dec. 2021) , art. 2106349  

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