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1.
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8 p, 4.8 MB |
Metal−organic frameworks : why make them small?
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Wang, Jiemin (Institut Català de Nanociència i Nanotecnologia) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Recent studies have demonstrated that metal−organic frameworks (MOFs) can be miniaturized down to the submicroscale and even nanoscale to create small MOFs. Herein, the basic concepts and recent progresses concerning the core question of "MOFs, why make them small?" are briefly introduced from three perspectives: those of size, shape, and processability. [...]
2022 -  10.1002/sstr.202100126
Small structures, Vol. 3, issue 1 (Jan. 2022) , art. 2100126
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2.
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12 p, 11.3 MB |
Influence of the surface chemistry of metal-organic polyhedra in their assembly into ultrathin films for gas separation
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Tejedor, Inés (Universidad de Zaragoza. Departamento de Química Física) ;
Andrés, Miguel A. (Instituto de Ciencia de Materiales de Aragón) ;
Carné-Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ;
Arjona, Mónica (Universidad de Zaragoza. Departamento de Química Física) ;
Pérez-Miana, Marta (Universidad de Zaragoza. Departamento de Ingeniería Química y Tecnologías del Medio Ambiente) ;
Sanchez-Lainez, Javier (Instituto de Nanociencia y Materiales de Aragón) ;
Coronas, Joaquin (Instituto de Nanociencia y Materiales de Aragón) ;
Fontaine, Philippe (Synchrotron SOLEIL) ;
Goldmann, Michel (Synchrotron SOLEIL) ;
Roubeau, Olivier (Instituto de Nanociencia y Materiales de Aragón) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Gascón, Ignacio (Universidad de Zaragoza. Departamento de Química Física)
The formation of ultrathin films of Rh-based porous metal-organic polyhedra (Rh-MOPs) by the Langmuir-Blodgett method has been explored. Homogeneous and dense monolayer films were formed at the air-water interface either using two different coordinatively alkyl-functionalized Rh-MOPs (HRhMOP(diz)and HRhMOP(oiz)) or by in situ incorporation of aliphatic chains to the axial sites of dirhodium paddlewheels of another Rh-MOP (OHRhMOP) at the air-liquid interface. [...]
2022 - 10.1021/acsami.2c06123
ACS applied materials & interfaces, Vol. 14, issue 23 (June 2022) , p. 27495-27506
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3.
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8 p, 4.8 MB |
Ammonia capture in rhodium(II)-based metal-organic polyhedra via synergistic coordinative and H-bonding interactions
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Carné-Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ;
Martínez-Esaín, Jordi (Institut Català de Nanociència i Nanotecnologia) ;
Rookard, Tanner (Oregon State University. Department of Chemistry) ;
Flood, Christopher J. (Oregon State University. Department of Chemistry) ;
Faraudo, Jordi (Institut de Ciència de Materials de Barcelona) ;
Stylianou, Kyriakos C (Oregon State University. Department of Chemistry) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Ammonia (NH) is among the world's most widely produced bulk chemicals, given its extensive use in diverse sectors such as agriculture; however, it poses environmental and health risks at low concentrations. [...]
2023 - 10.1021/acsami.2c19206
ACS applied materials & interfaces, Vol. 15, issue 5 (Feb. 2023) , p. 6747-6754
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4.
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5.
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14 p, 4.2 MB |
Perspectives for polychlorinated trityl radicals
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Ratera Bastardas, Imma (Institut de Ciència de Materials de Barcelona) ;
Vidal-Gancedo, José (Institut de Ciència de Materials de Barcelona) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Bromley, Stefan (Universitat de Barcelona. Departament de Ciència de Materials i Química Física) ;
Crivillers, Núria (Institut de Ciència de Materials de Barcelona) ;
Mas-Torrent, Marta (Institut de Ciència de Materials de Barcelona)
An organic free radical is a molecule with one or more unpaired electrons. Although most free radicals are highly reactive, chemists have developed a few families of so-called persistent organic radicals with high kinetic stabilities. [...]
2021 - 10.1039/d1tc02196f
Journal of Materials Chemistry C, Vol. 9, issue 33 (Sep. 2021) , p. 10610-10623
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6.
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8 p, 2.8 MB |
Coloration in supraparticles assembled from polyhedral metal-organic framework particles
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Wang, Junwei (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Particle Technology) ;
Liu, Yang (Institut Català de Nanociència i Nanotecnologia) ;
Bleyer, Gudrun (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Particle Technology) ;
Goerlitzer, Eric S. A. (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Particle Technology) ;
Englisch, Silvan (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Micro- and Nanostructure Research) ;
Przybilla, Thomas (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Micro- and Nanostructure Research) ;
Mbah Chrameh, Fru (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute for Multiscale Simulation) ;
Engel, Michael (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute for Multiscale Simulation) ;
Spiecker, Erdmann (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Micro- and Nanostructure Research) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Vogel, Nicolas (Friedrich-Alexander Universität Erlangen-Nürnberg. Institute of Particle Technology)
Supraparticles are spherical colloidal crystals prepared by confined self-assembly processes. A particularly appealing property of these microscale structures is the structural color arising from interference of light with their building blocks. [...]
2022 - 10.1002/anie.202117455
Angewandte Chemie, Vol. 61, issue 16 (April 2022) , art. e202117455
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7.
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13 p, 4.0 MB |
Antibacterial films based on MOF composites that release iodine passively or upon triggering by near-infrared light
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Han, Xu (Institut Català de Nanociència i Nanotecnologia) ;
Boix, Gerard (Institut Català de Nanociència i Nanotecnologia) ;
Balcerzak, Mateusz (Institut Català de Nanociència i Nanotecnologia) ;
Moriones, Oscar Hernando (Universitat Autònoma de Barcelona) ;
Cano-Sarabia, Mary (Institut Català de Nanociència i Nanotecnologia) ;
Cortés Garmendia, M. Pilar (Universitat Autònoma de Barcelona. Departament de Genètica i de Microbiologia) ;
Bastús, Neus G. (Institut Català de Nanociència i Nanotecnologia) ;
Puntes, Víctor (Institut Català de Nanociència i Nanotecnologia) ;
Llagostera Casas, Montserrat (Universitat Autònoma de Barcelona. Departament de Genètica i de Microbiologia) ;
Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Boix, Gerard (Institut Català de Nanociència i Nanotecnologia)
Multidrug-resistant bacteria have become a global health problem for which new prophylactic strategies are now needed, including surface-coatings for hospital spaces and medical equipment. This work reports the preparation and functional validation of a metal-organic framework (MOF) based composite for the triggered controlled release of iodine, an antimicrobial element that does not generate resistance. [...]
2022 - 10.1002/adfm.202112902
Advanced functional materials, Vol. 32, issue 19 (May 2022) , art. 2112902
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8.
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12 p, 4.7 MB |
Surface chemistry of metal-organic polyhedra
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Albalad, Jorge (The University of Adelaide. Department of Chemistry) ;
Hernández López, Laura (Institut Català de Nanociència i Nanotecnologia) ;
Carné-Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Metal-organic polyhedra (MOPs) are discrete, intrinsically-porous architectures that operate at the molecular regime and, owing to peripheral reactive sites, exhibit rich surface chemistry. Researchers have recently exploited this reactivity through post-synthetic modification (PSM) to generate specialised molecular platforms that may overcome certain limitations of extended porous materials. [...]
2022 - 10.1039/d1cc07034g
Chemical communications, Vol. 58, issue 15 (Feb 2022) , p. 2443-2454
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9.
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9 p, 1.8 MB |
pH-triggered removal of nitrogenous organic micropollutants from water by using metal-organic polyhedra
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Hernández-López, Laura (Institut Català de Nanociència i Nanotecnologia) ;
Cortés-Martínez, Alba (Universitat Autònoma de Barcelona. Departament de Química) ;
Parella Coll, Teodor (Universitat Autònoma de Barcelona. Servei de Ressonància Magnètica Nuclear) ;
Carné-Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Water pollution threatens human and environmental health worldwide. Thus, there is a pressing need for new approaches to water purification. Herein, we report a novel supramolecular strategy based on the use of a metal-organic polyhedron (MOP) as a capture agent to remove nitrogenous organic micropollutants from water, even at very low concentrations (ppm), based exclusively on coordination chemistry at the external surface of the MOP. [...]
2022 - 10.1002/chem.202200357
Chemistry, Vol. 28, issue 31 (June 2022) , art. e202200357
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10.
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12 p, 1.6 MB |
How reproducible are surface areas calculated from the BET equation?
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Osterrieth, Johannes W. M. (University of Cambridge. Department of Chemical Engineering & Biotechnology) ;
Rampersad, James (University of Cambridge. Department of Chemical Engineering & Biotechnology) ;
Madden, David (University of Cambridge. Department of Chemical Engineering & Biotechnology) ;
Rampal, Nakul (University of Cambridge. Department of Chemical Engineering & Biotechnology) ;
Skoric, Luka (University of Cambridge. Cavendish Laboratory) ;
Connolly, Bethany (University of Cambridge. Department of Chemical Engineering & Biotechnology) ;
Allendorf, Mark D. (Sandia National Laboratories) ;
Stavila, Vitalie (Sandia National Laboratories) ;
Snider, Jonathan L. (Sandia National Laboratories) ;
Ameloot, Rob (KU Leuven. Department of Microbial and Molecular Systems) ;
Marreiros, Joao (KU Leuven. Department of Microbial and Molecular Systems) ;
Ania, Conchi (Université d'Orléans) ;
Azevedo, Diana (Federal University of Ceará. Department of Chemical Engineering) ;
Vilarrasa-Garcia, Enrique (Federal University of Ceará. Department of Chemical Engineering) ;
Santos, Bianca F. (Federal University of Ceará. Department of Chemical Engineering) ;
Bu, Xian-He (Nankai University. School of Materials Science and Engineering) ;
Chang, Ze (Nankai University. School of Materials Science and Engineering) ;
Bunzen, Hana (University of Augsburg. Institute of Physics) ;
Champness, Neil R. (University of Nottingham. School of Chemistry) ;
Griffin, Sarah L. (University of Nottingham. School of Chemistry) ;
Chen, Banglin (University of Texas at San Antonio. Department of Chemistry) ;
Lin, Rui-Biao (University of Texas at San Antonio. Department of Chemistry) ;
Coasne, Benoit (Université Grenoble Alpes) ;
Cohen, Seth (University of California. Department of Chemistry and Biochemistry) ;
Moreton, Jessica C. (University of California. Department of Chemistry and Biochemistry) ;
Colón, Yamil J. (Université de Nôtre Dame) ;
Chen, Linjiang (Leverhulme Research Centre for Functional Materials Design) ;
Clowes, Rob (Leverhulme Research Centre for Functional Materials Design) ;
Coudert, François-Xavier (Chimie ParisTech) ;
Cui, Y. (Shanghai Jiaotong University. School of Chemistry and Chemical Engineering) ;
Hou, B. (Shanghai Jiaotong University. School of Chemistry and Chemical Engineering) ;
D'Alessandro, D.M. (The University of Sydney. School of Chemistry) ;
Doheny, P.W. (The University of Sydney. School of Chemistry) ;
Dincă, M. (Massachusetts Institute of Technology. Department of Chemistry) ;
Sun, C. (Massachusetts Institute of Technology. Department of Chemistry) ;
Doonan, C. (The University of Adelaide. Centre for Advanced Nanomaterials and Department of Chemistry) ;
Huxley, M.T. (The University of Adelaide. Centre for Advanced Nanomaterials and Department of Chemistry) ;
Evans, J.D. (Technische Universität Dresden. Department of Inorganic Chemistry) ;
Falcaro, P. (Graz University of Technology. Institute of Physical and Theoretical Chemistry) ;
Ricco, R. (Graz University of Technology. Institute of Physical and Theoretical Chemistry) ;
Farha, O. (Northwestern University. Department of Chemistry) ;
Idrees, K.B. (Northwestern University. Department of Chemistry) ;
Islamoglu, T. (Northwestern University. Department of Chemistry) ;
Feng, P. (University of California. Department of Chemistry) ;
Yang, H. (University of California. Department of Chemistry) ;
Forgan, R.S. (University of Glasgow. School of Chemistry) ;
Bara, D. (University of Glasgow. School of Chemistry) ;
Furukawa, Shuhei (Kyoto University. Institute for Integrated Cell-Material Sciences) ;
Sanchez, E. (Kyoto University. Institute for Integrated Cell-Material Sciences) ;
Gascon, J. (KAUST Catalysis Center) ;
Telalović, S. (KAUST Catalysis Center) ;
Ghosh, S.K. (Indian Institute of Science Education and Research. Department of Chemistry) ;
Mukherjee, S. (Indian Institute of Science Education and Research. Department of Chemistry) ;
Hill, Matthew R (Monash University. Department of Chemical Engineering) ;
Sadiq, M.M. (Monash University. Department of Chemical Engineering) ;
Horcajada, P. (IMDEA Energy) ;
Salcedo-Abraira, P. (IMDEA Energy) ;
Kaneko, K. (Shinshu University. Research Initiative for Supra-Materials) ;
Kukobat, R. (Shinshu University. Research Initiative for Supra-Materials) ;
Kenvin, J. (Micromeritics Instrument Corporation) ;
Keskin, S. (Koc University. Department of Chemical and Biological Engineering) ;
Kitagawa, S. (Kyoto University Institute for Advanced Study) ;
Otake, K.i. (Kyoto University Institute for Advanced Study) ;
Lively, R.P. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
DeWitt, S.J.A. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
Llewellyn, P. (CNRS / Aix-Marseille Univ./Total) ;
Lotsch, B.V. (University of Munich. Department of Chemistry) ;
Emmerling, S.T. (University of Munich. Department of Chemistry) ;
Pütz, A.M. (University of Munich. Department of Chemistry) ;
Martí-Gastaldo, C. (Universitat de València. Instituto de Ciencia Molecular) ;
Padial, Natalia M (Universitat de València. Instituto de Ciencia Molecular) ;
García-Martínez, J. (Universitat d'Alacant. Laboratori de Nanotecnologia Molecular) ;
Linares, N. (Universitat d'Alacant. Laboratori de Nanotecnologia Molecular) ;
Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia) ;
Suárez del Pino, José A. (Institut Català de Nanociència i Nanotecnologia) ;
Moghadam, P. (The University of Sheffield. Department of Chemical and Biological Engineering) ;
Oktavian, R. (The University of Sheffield. Department of Chemical and Biological Engineering) ;
Morris, R.E. (University of St Andrews. School of Chemistry) ;
Wheatley, P.S. (University of St Andrews. School of Chemistry) ;
Navarro, J. (Universidad de Granada) ;
Petit, C. (Barrer Centre) ;
Danaci, D. (Barrer Centre) ;
Rosseinsky, M.J. (University of Liverpool. Department of Chemistry) ;
Katsoulidis, A.P. (University of Liverpool. Department of Chemistry) ;
Schröder, M. (The University of Manchester. School of Chemistry) ;
Han, X. (The University of Manchester. School of Chemistry) ;
Yang, S. (The University of Manchester. School of Chemistry) ;
Serre, C. (Institut des Matériaux Poreux de Paris) ;
Mouchaham, G. (Institut des Matériaux Poreux de Paris) ;
Sholl, D.S. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
Thyagarajan, R. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
Siderius, D. (Chemical Sciences Division. National Institute of Standards and Technology) ;
Snurr, R.Q. (Northwestern University. Department of Chemical & Biological Engineering) ;
Goncalves, R.B. (Northwestern University. Department of Chemistry) ;
Telfer, S. (MacDiarmid Institute for Advanced Materials and Nanotechnology) ;
Lee, S.J. (MacDiarmid Institute for Advanced Materials and Nanotechnology) ;
Ting, V.P. (University of Bristol. Department of Mechanical Engineering) ;
Rowlandson, J.L. (University of Bristol. Department of Mechanical Engineering) ;
Uemura, T. (The University of Tokyo. Department of Advanced Materials Science) ;
Iiyuka, T. (The University of Tokyo. Department of Advanced Materials Science) ;
van der Veen, M.A. (Delft University of Technology. Department of Chemical Engineering) ;
Rega, D. (Delft University of Technology. Department of Chemical Engineering) ;
Van Speybroeck, V. (Ghent University. Center for Molecular Modeling) ;
Rogge, S.M.J. (Ghent University. Center for Molecular Modeling) ;
Lamaire, A. (Ghent University. Center for Molecular Modeling) ;
Walton, K.S. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
Bingel, L.W. (Georgia Institute of Technology. School of Chemical & Biomolecular Engineering) ;
Wuttke, S. (IKERBASQUE) ;
Andreo, J. (IKERBASQUE) ;
Yaghi, O. (Berkeley Global Science Institute) ;
Zhang, B. (University of California. Department of Chemistry) ;
Yavuz, C.T. (Korea Advanced Institute of Science and Technology) ;
Nguyen, T.S. (Korea Advanced Institute of Science and Technology) ;
Zamora, Félix (Universidad Autónoma de Madrid. Departamento de Química Inorgánica) ;
Montoro, C. (Universidad Autónoma de Madrid. Departamento de Química Inorgánica) ;
Zhou, H. (Texas A&M University. Department of Chemistry) ;
Kirchon, A. (Texas A&M University. Department of Chemistry) ;
Fairen-Jimenez, D. (University of Cambridge. Department of Chemical Engineering & Biotechnology)
Porosity and surface area analysis play a prominent role in modern materials science. At the heart of this sits the Brunauer-Emmett-Teller (BET) theory, which has been a remarkably successful contribution to the field of materials science. [...]
2022 - 10.1002/adma.202201502
Advanced materials, Vol. 34, issue 27 (July 2022) , art. 2201502
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