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11 p, 3.1 MB C-H Amination Reactions Mediated by Metastable Pseudo- O Masked Aryl-Co III -nitrene Species / Capdevila, Lorena (Universitat de Girona. Departament de Química) ; Montilla, Marc (Universitat de Girona. Departament de Química) ; Planas, Oriol (Universitat de Girona. Departament de Química) ; Brotons, Artur (Universitat de Girona. Departament de Química) ; Salvador, Pedro (Universitat de Girona. Departament de Química) ; Martin-Diaconescu, Vlad (ALBA Laboratori de Llum de Sincrotró) ; Parella Coll, Teodor (Universitat Autònoma de Barcelona. Servei de Ressonància Magnètica Nuclear) ; Luis, Josep M. (Universitat de Girona. Departament de Química) ; Ribas, Xavi (Universitat de Girona. Departament de Química)
Cobalt-catalyzed C-H amination via M-nitrenoid species is spiking the interest of the research community. Understanding this process at a molecular level is a challenging task, and here we report a well-defined macrocyclic system featuring a pseudo- O aryl-Co III species that reacts with aliphatic azides to effect intramolecular C-N bond formation. [...]
2022 - 10.1021/acs.inorgchem.2c02111
Inorganic chemistry, Vol. 61, Issue 35 (August 2022) , p. 14075-14085  
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