Depósito Digital de Documentos de la UAB Encontrados 5 registros  La búsqueda tardó 0.01 segundos. 
1.
11 p, 1.2 MB Influence of the Amide Groups in the CO2/N2 Selectivity of a Series of Isoreticular, Interpenetrated Metal-Organic Frameworks / Safarifard, Vahid (Institut Català de Nanociència i Nanotecnologia) ; Rodríguez-Hermida, Sabina (Institut Català de Nanociència i Nanotecnologia) ; Guillerm, Vincent (Institut Català de Nanociència i Nanotecnologia) ; Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ; Bigdeli, Mina (Tarbiat Modares University. Department of Chemistry) ; Tehrani, Alireza Azhdari (Tarbiat Modares University. Department of Chemistry) ; Juanhuix, Jordi (ALBA Laboratori de Llum de Sincrotró) ; Morsali, Ali (Tarbiat Modares University. Department of Chemistry) ; Casco, Mirian E. (Universidad de Alicante. Departamento de Química Inorgánica) ; Silvestre Albero, Joaquín (Universidad de Alicante. Departamento de Química Inorgánica) ; Ramos Fernández, Enrique V. (Universidad de Alicante. Departamento de Química Inorgánica) ; Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Here we report the use of a pillaring strategy for the design and synthesis of three novel amide-functionalized metal-organic frameworks (MOFs), TMUs-22/-23/-24, isoreticular to the recently reported imine-functionalized TMU-6 and TMU-21 MOFs. [...]
2016 - 10.1021/acs.cgd.6b01054
Crystal Growth and Design, Vol. 16, Issue 10 (October 2016) , p. 6016-6023  
2.
9 p, 962.7 KB Optimised room temperature, water-based synthesis of CPO-27-M metal-organic frameworks with high space-time yields / Garzón Tovar, Luis (Institut Català de Nanociència i Nanotecnologia) ; Carné Sánchez, Arnau (Institut Català de Nanociència i Nanotecnologia) ; Carbonell Fernández, Carlos (Institut Català de Nanociència i Nanotecnologia) ; Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ; Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
The exceptional porosity of Metal-Organic Frameworks (MOFs) could be harnessed for countless practical applications. However, one of the challenges currently precluding the industrial exploitation of these materials is a lack of green methods for their synthesis. [...]
2015 - 10.1039/c5ta04923g
Journal of materials chemistry A, Vol. 3, Issue 41 (November 2015) , p. 20819-20826  
3.
17 p, 1.2 MB Postsynthetic Selective Ligand Cleavage by Solid-Gas Phase Ozonolysis Fuses Micropores into Mesopores in Metal-Organic Frameworks / Guillerm, Vincent (Institut Català de Nanociència i Nanotecnologia) ; Xu, Heng (Institut Català de Nanociència i Nanotecnologia) ; Albalad, Jorge (Institut Català de Nanociència i Nanotecnologia) ; Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ; Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Herein we report a novel, ozone-based method for postsynthetic generation of mesoporosity in metal-organic frameworks (MOFs). By carefully selecting mixed-ligand Zr-fcu-MOFs based on organic ligand pairs in which one ligand has ozone-cleavable olefin bonds and the other ligand is ozone-resistant, we were able to selectively break the cleavable ligand via ozonolysis to trigger fusion of micropores into mesopores within the MOF framework. [...]
2018 - 10.1021/jacs.8b09682
Journal of the American Chemical Society, Vol. 140, Issue 44 (November 2018) , p. 15022-15030  
4.
6 p, 767.9 KB Zigzag ligands for transversal design in reticular chemistry : unveiling new structural opportunities for metal-organic frameworks / Guillerm, Vincent (Institut Català de Nanociència i Nanotecnologia) ; Grancha, Thais (Institut Català de Nanociència i Nanotecnologia) ; Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ; Juanhuix, Judith (ALBA Laboratori de Llum de Sincrotró) ; Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Herein we describe the topological influence of zigzag ligands in the assembly of Zr(IV) metal-organic frameworks (MOFs). Through a transversal design strategy using reticular chemistry, we were able to synthesize a family of isoreticular Zr(IV)-based MOFs exhibiting the bcu - rather than the fcu - topology. [...]
2018 - 10.1021/jacs.8b07050
Journal of the American Chemical Society, Vol. 140, issue 32 (August 2018) , p. 10153-10157  
5.
23 p, 959.0 KB Spray drying for making covalent chemistry : postsynthetic modification of metal-organic frameworks / Garzón Tovar, Luis (Institut Català de Nanociència i Nanotecnologia) ; Rodríguez-Hermida, Sabina (Institut Català de Nanociència i Nanotecnologia) ; Imaz, Inhar (Institut Català de Nanociència i Nanotecnologia) ; Maspoch Comamala, Daniel (Institut Català de Nanociència i Nanotecnologia)
Covalent postsynthetic modification (PSM) of metal-organic frameworks (MOFs) has attracted much attention due to the possibility of tailoring the properties of these porous materials. Schiff-base condensation betwecn an amine and an aldehyde is one of the most common reactions in the PSM of MOFs. [...]
2017 - 10.1021/jacs.6b11240
Journal of the American Chemical Society, Vol. 139, Núm. 2 (January 2017) , p. 897-903
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