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12 p, 2.1 MB Enabling full-scale grain boundary mitigation in polycrystalline perovskite solids / Zhao, Lichen (Peking University. State Key Laboratory for Artificial Microstructure and Mesoscopic Physics) ; Tang, PengYi (Institut Català de Nanociència i Nanotecnologia) ; Luo, Deying (Peking University. State Key Laboratory for Artificial Microstructure and Mesoscopic Physics) ; Dar, Ibrahim (University of Cambridge. Department of Physics) ; Eickemeyer, Felix (École Polytechnique Fédérale de Lausanne. Laboratory of Photonics and Interfaces) ; Arora, Neha (University of Cambridge. Department of Physics) ; Hu, Qin (University of Massachusetts. Polymer Science and Engineering Department) ; Luo, Jingshan (École Polytechnique Fédérale de Lausanne. Laboratory of Photonics and Interfaces) ; Liu, Yuhang (École Polytechnique Fédérale de Lausanne. Laboratory of Photonics and Interfaces) ; Zakeeruddin, Shaik Mohammed (École Polytechnique Fédérale de Lausanne. Laboratory of Photonics and Interfaces) ; Hagfeldt, Anders (École Polytechnique Fédérale de Lausanne. Laboratory of Photomolecular Science) ; Arbiol i Cobos, Jordi (Institut Català de Nanociència i Nanotecnologia) ; Huang, Wei (Nanjing Tech University. Key Laboratory of Flexible Electronics & Institute of Advanced Materials) ; Gong, Qihuang (Peking University. State Key Laboratory for Artificial Microstructure and Mesoscopic Physics) ; Russell, Thomas (University of Massachusetts. Polymer Science and Engineering Department) ; Friend, Richard Henry (University of Cambridge. Department of Physics) ; Grätzel, Michael (École Polytechnique Fédérale de Lausanne. Laboratory of Photonics and Interfaces) ; Zhu, Rui (Peking University. State Key Laboratory for Artificial Microstructure and Mesoscopic Physics)
There exists a considerable density of interaggregate grain boundaries (GBs) and intra-aggregate GBs in polycrystalline perovskites. Mitigation of intra-aggregate GBs is equally notable to that of interaggregate GBs as intra-aggregate GBs can also cause detrimental effects on the photovoltaic performances of perovskite solar cells (PSCs). [...]
2022 - 10.1126/sciadv.abo3733
Science advances, Vol. 8, issue 35 (Sep. 2022) , art. eabo3733  
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