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10 p, 2.0 MB Cyclobutene vs 1,3-Diene Formation in the Gold-Catalyzed Reaction of Alkynes with Alkenes : The Complete Mechanistic Picture / Orbe, M. Elena de (Institut Català d'Investigació Química) ; Amenós, Laura (Institut Català d'Investigació Química) ; Kirillova, Mariia S. (Institut Català d'Investigació Química) ; Wang, Yahui (Institut Català d'Investigació Química) ; López Carrillo, Verónica (Institut Català d'Investigació Química) ; Maseras Cuní, Feliu (Universitat Autònoma de Barcelona. Departament de Química) ; Echavarren, Antonio M. (Universitat Rovira i Virgili)
The intermolecular gold(I)-catalyzed reaction between arylalkynes and alkenes leads to cyclobutenes by a [2 + 2] cycloaddition, which takes place stepwise, first by formation of cyclopropyl gold(I) carbenes, followed by a ring expansion. [...]
2017 - 10.1021/jacs.7b03005
Journal of the American Chemical Society, Vol. 139, Issue 30 (August 2017) , p. 10302-10311  
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