Misfit Dislocation Guided Topographic and Conduction Patterning in Complex Oxide Epitaxial Thin Films
Sandiumenge Ortiz, Felip 
(Institut de Ciència de Materials de Barcelona)
Bagués Salgueró, Núria 
(Institut Català de Nanociència i Nanotecnologia)
Santiso, José 
(Institut Català de Nanociència i Nanotecnologia)
Paradinas Aranjuelo, Marcos 
(Institut Català de Nanociència i Nanotecnologia)
Pomar, Alberto 
(Institut de Ciència de Materials de Barcelona)
Konstantinovic, Zorica (University of Belgrade)
Ocal García, Carmen
(Institut de Ciència de Materials de Barcelona)
Balcells Argemí, Lluís
(Institut de Ciència de Materials de Barcelona)
Casanove, Marie-Jo (Universite de Toulouse)
Martínez, Benjamín
(Institut de Ciència de Materials de Barcelona)
Date: |
2016 |
Abstract: |
Interfacial dissimilarity has emerged in recent years as the cornerstone of emergent interfacial phenomena, while enabling the control of electrical transport and magnetic behavior of complex oxide epitaxial films. As a step further toward the lateral miniaturization of functional nanostructures, this work uncovers the role of misfit dislocations in creating periodic surface strain patterns that can be efficiently used to control the spatial modulation of mass transport phenomena and bandwidth-dependent properties on a ≈20 nm length scale. The spontaneous formation of surface strain-relief patterns in LaSrMnO/LaAlO films results in lateral periodic modulations of the surface chemical potential and tetragonal distortion, controlling the spatial distribution of preferential nucleation sites and the bandwidth of the epilayer, respectively. These results provide insights into the spontaneous formation of strain-driven ordered surface patterns, topographic and functional, during the growth of complex oxide heterostructures on lengths scales far below the limits achievable through top-down approaches. |
Note: |
Número d'acord de subvenció MINECO/SEV-2015-0496 |
Note: |
Número d'acord de subvenció MINECO/MAT2015-71664-R |
Note: |
Número d'acord de subvenció MINECO/MAT2012-33207 |
Note: |
Número d'acord de subvenció MINECO/MAT2013-47869-C4-1-P |
Note: |
Número d'acord de subvenció EC/H2020/645658 |
Note: |
Número d'acord de subvenció AGAUR/2014/SGR-501 |
Note: |
Número d'acord de subvenció EC/FP7/312483 |
Rights: |
Tots els drets reservats.  |
Language: |
Anglès |
Document: |
article ; recerca ; acceptedVersion |
Subject: |
Complex oxides ;
Misfit dislocations ;
Strain ;
Surface current ;
Surface patterning |
Published in: |
Advanced materials interfaces, Vol. 3, Issue 14 (July 2016) , art. 1600106, ISSN 2196-7350 |
DOI: 10.1002/admi.201600106
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Record created 2019-07-30, last modified 2020-08-02