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Chitin nanofiber paper toward optical (bio)sensing applications
Naghdi, Tina (Institut Català de Nanociència i Nanotecnologia)
Golmohammadi, Hamed (Chemistry and Chemical Engineering Research Center of Iran)
Yousefi, Hossein (Gorgan University of Agricultural Sciences and Natural Resources. Department of Wood Engineering and Technology)
Hosseinifard, Mohammad (Chemistry and Chemical Engineering Research Center of Iran)
Kostiv, Uliana (Academy of Sciences of the Czech Republic. Institute of Macromolecular Chemistry)
Horák, Daniel (Academy of Sciences of the Czech Republic. Institute of Macromolecular Chemistry)
Merkoçi, Arben (Institut Català de Nanociència i Nanotecnologia)

Data: 2020
Resum: Because of numerous inherent and unrivaled features of nanofibers made of chitin, the second most plentiful natural-based polymer (after cellulose), including affordability, abundant nature, biodegradability, biocompatibility, commercial availability, flexibility, transparency, and extraordinary mechanical and physicochemical properties, chitin nanofibers (ChNFs) are being applied as one of the most appealing bionanomaterials in a myriad of fields. Herein, we exploited the beneficial properties offered by the ChNF paper to fabricate transparent, efficient, biocompatible, flexible, and miniaturized optical sensing bioplatforms via embedding/immobilizing various plasmonic nanoparticles (silver and gold nanoparticles), photoluminescent nanoparticles (CdTe quantum dots, carbon dots, and NaYF:Yb@Er&SiO upconversion nanoparticles) along with colorimetric reagents (curcumin, dithizone, etc. ) in the 3D nanonetwork scaffold of the ChNF paper. Several configurations, including 2D multi-wall and 2D cuvette patterns with hydrophobic barriers/walls and hydrophilic test zones/channels, were easily printed using laser printing technology or punched as spot patterns on the dried ChNF paper-based nanocomposites to fabricate the (bio)sensing platforms. A variety of (bio)chemicals as model analytes were used to confirm the efficiency and applicability of the fabricated ChNF paper-based sensing bioplatforms. The developed (bio)sensors were also coupled with smartphone technology to take the advantages of smartphone-based monitoring/sensing devices along with the Internet of Nano Things (IoNT)/the Internet of Medical Things (IoMT) concepts for easy-to-use sensing applications. Building upon the unrivaled and inherent features of ChNF as a very promising bionanomaterial, we foresee that the ChNF paper-based sensing bioplatforms will emerge new opportunities for the development of innovative strategies to fabricate cost-effective, simple, smart, transparent, biodegradable, miniaturized, flexible, portable, and easy-to-use (bio)sensing/monitoring devices.
Ajuts: Ministerio de Economía y Competitividad SEV-2017-0706
Ministerio de Economía y Competitividad MAT2017-87202-P
Nota: Altres ajuts: The ICN2 is funded by the CERCA Programme/Generalitat de Catalunya. The financial support of "the Czech Science Foundation (No. 19-00676S)" is also greatly appreciated.
Drets: Tots els drets reservats.
Llengua: Anglès
Document: Article ; recerca ; Versió sotmesa a revisió
Publicat a: ACS applied materials & interfaces, Vol. 12, issue 13 (April 2020) , p. 15538-15552, ISSN 1944-8252

DOI: 10.1021/acsami.9b23487


Preprint
46 p, 2.3 MB

El registre apareix a les col·leccions:
Documents de recerca > Documents dels grups de recerca de la UAB > Centres i grups de recerca (producció científica) > Ciències > Institut Català de Nanociència i Nanotecnologia (ICN2)
Articles > Articles de recerca
Articles > Articles publicats

 Registre creat el 2021-01-25, darrera modificació el 2023-10-01



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