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Molecular engineering to introduce carbonyl between nickel salophen active sites to enhance electrochemical CO2 reduction to methanol / Liang, Zhifu (Institut Català de Nanociència i Nanotecnologia) ; Wang, Jianghao (Institute of Zhejiang University) ; Tang, PengYi (Peter Grünberg Institute Forschungszentrum Jülich GmbH) ; Tang, Weiqiang (East China University of Science and Technology) ; Liu, Lijia (Western University. Department of Chemistry) ; Shakouri, Mohsen (Canadian Light Source) ; Wang, Xiang (Institut de Recerca en Energia de Catalunya) ; Llorca, Jordi (Universitat Politècnica de Catalunya. Institut de Tècniques Energètiques) ; Zhao, Shuangliang (Guangxi University. School of Chemistry and Chemical Engineering) ; Heggen, Marc (Peter Grünberg Institute Forschungszentrum Jülich GmbH) ; Dunin-Borkowski, Rafal E. (Peter Grünberg Institute Forschungszentrum Jülich GmbH) ; Cabot, Andreu (Institució Catalana de Recerca i Estudis Avançats) ; Wu, Hao Bin (Zhejiang University. School of Materials Science and Engineering) ; Arbiol i Cobos, Jordi (Institut Català de Nanociència i Nanotecnologia)
The electrochemical reduction of CO to methanol is a potentially cost-effective strategy to reduce the concentration of this greenhouse gas while at the same time producing a value-added chemical. Herein, we detail a highly efficient 2D nickel organic framework containing a large density of highly dispersed salophen NiNO active sites toward electrochemical CORR to methanol. [...]
2022 - DOI (Digital Object Identifier)

10.1016/j.apcatb.2022.121451
Applied catalysis. B, Environmental, Vol. 314 (Oct. 2022) , art. 121451

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