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| Pàgina inicial > Articles > Articles publicats > Thermal conductivity of MoS2 polycrystalline nanomembranes |
| Data: | 2016 |
| Resum: | Heat conduction in 2D materials can be effectively engineered by means of controlling nanoscale grain structure. Afavorable thermal performance makes these structures excellent candidates for integrated heat management units. Here we show combined experimental and theoretical studies for MoS₂ nanosheets in a nanoscale grain-size limit. Wereport thermal conductivity measurements on 5 nm thick polycrystalline MoS₂ by means of 2-laser Raman thermometry. The free-standing, drum-like MoS₂ nanomembranes were fabricated using a novel polymer- and residue-free, wet transfer, in which we took advantage of the difference in the surface energies between MoS₂ and the growth substrate to transfer the CVD-grown nanosheets. The measurements revealed a strong reduction in the in-plane thermal conductivity down to about 0. 73 ± 0. 25 W m⁻¹ K⁻¹. The results are discussed theoretically using finite elements method simulations for a polycrystalline film, and a scaling trend of the thermally conductivity with grain size is proposed. |
| Ajuts: | European Commission 604668 European Commission 309150 Ministerio de Ciencia e Innovación SEV-2013-0295 Ministerio de Ciencia e Innovación MAT2012-31392 Ministerio de Ciencia e Innovación CSD2010-0044 |
| Drets: | Aquest document està subjecte a una llicència d'ús Creative Commons. Es permet la reproducció total o parcial, la distribució, i la comunicació pública de l'obra, sempre que no sigui amb finalitats comercials, i sempre que es reconegui l'autoria de l'obra original. No es permet la creació d'obres derivades. |
| Llengua: | Anglès |
| Document: | Article ; recerca ; Versió acceptada per publicar |
| Matèria: | Nanoscale thermal transport ; Thermal conductivity ; Ultra-thin membranes |
| Publicat a: | 2D materials, Vol. 3, no. 3 (Sep. 2016) , art. 35016, ISSN 2053-1583 |
Postprint 10 p, 908.2 KB |